Sökning: "ultrafast dissociation"
Visar resultat 1 - 5 av 10 avhandlingar innehållade orden ultrafast dissociation.
1. Ultrafast Probing of CO Reactions on Metal Surfaces : Changes in the molecular orbitals during the catalysis process
Sammanfattning : This thesis presents experimental studies of three different chemical reaction steps relevant for heterogeneous catalysis: dissociation, desorption, and oxidation. CO on single-crystal metal surfaces was chosen as the model systems. LÄS MER
2. Ultrafast Photoionization Dynamics Studied with Coincidence Momentum Imaging Spectrometers
Sammanfattning : The time scale of the dynamics in atoms and molecules varies from attoseconds (10-18) to picoseconds (10-12) depending on the size of the particles. To study such dynamics, ultrafast light pulses are needed to trigger and capture the reaction. One of the most direct methods consists in ionizing the system and observing the following response. LÄS MER
3. Studies of Ultrafast Relaxation and Photodissociation Processes in Solution
Sammanfattning : This thesis focuses on femtosecond studies of relaxation and photo-induced dissociation processes in the liquid environment. Measurements are performed using both polarization sensitive and magic angle transient absorption spectroscopy with excitation wavelengths of 387 nm and 258 nm and a white light continuum probe. LÄS MER
4. Multimode resonant X-ray scattering of free molecules
Sammanfattning : This thesis is focused on the role that nuclear dynamics plays in the formation of X-ray absorption (XAS) and resonant inelastic X-ray scattering (RIXS) spectra of multimode free molecules. A combined approach based on ab initio electronic structure methods and quantum nuclear wave packet dynamics is applied to two systems -- water and methanol in the gas phase. LÄS MER
5. Characterization of Ultrashort Pulses And Ultrafast Dynamics of Molecules In the Liquid Phase
Sammanfattning : This thesis reports an alternative method for fully acomplete characterization of the UV pump pulse and white lightcontinuum probe pulse, which is commonly used in the pump-probeexperiments to investigate the ultrafast dynamics of molecules.Besides that, real dynamics of infrared cyanine dye molecules(Methyl-DOTCI) and photo-induced dissociation of trihalide ions(I3-or I2Br-) solvated in different organic solvent has alsobeen carefully investigated. LÄS MER