Sökning: "single nanoparticle catalysis"

Visar resultat 1 - 5 av 12 avhandlingar innehållade orden single nanoparticle catalysis.

  1. 1. Nanofluidics as a tool for parallelized single nanoparticle characterization: Fluorescence single nanoparticle catalysis and size determination through 1D Brownian motion

    Författare :Sune Levin; Chalmers tekniska högskola; []
    Nyckelord :TEKNIK OCH TEKNOLOGIER; ENGINEERING AND TECHNOLOGY; NATURVETENSKAP; NATURAL SCIENCES; TEKNIK OCH TEKNOLOGIER; ENGINEERING AND TECHNOLOGY; NATURVETENSKAP; NATURAL SCIENCES; dark field microscopy; single nanoparticle catalysis; heterogenous catalysis; particle tracking; Brownian motion; fluorescence microscopy; nanofluidics;

    Sammanfattning : Nanoparticles exist widely in nature and are objects of study in many scientific disciplines due to their high performance in a wide range of applications. With modern techniques that facilitate creating and shaping of nanoparticles into ever more complex shapes and compositions, characterization of particle properties is essential. LÄS MER

  2. 2. Nanofluidic Scattering Microscopy for Single Particle Catalysis

    Författare :Björn Altenburger; Chalmers tekniska högskola; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; NATURVETENSKAP; NATURAL SCIENCES; NATURVETENSKAP; NATURAL SCIENCES; label-free methods; Platinum; Nanofluidics; Single nanoparticle catalysis; Particle trapping; Hydrogen Peroxide decomposition; Colloidal particles; Dark field microscopy;

    Sammanfattning : Heterogeneous catalysis concerns material formulations – catalysts – that can assist a chemical reaction by improving its rate or selectivity, by lowering activation barriers and altering the energy landscape. The core of catalysts are often tiny metal particles that provide a large reaction surface at a small volume, as well as low coordination sites whose type and abundance depends on particle size and shape. LÄS MER

  3. 3. Operando Single Particle Catalysis - Combining a Nanoreactor and Plasmonic Nanospectroscopy

    Författare :David Albinsson; Chalmers tekniska högskola; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; NATURVETENSKAP; NATURAL SCIENCES; TEKNIK OCH TEKNOLOGIER; ENGINEERING AND TECHNOLOGY; NATURVETENSKAP; NATURAL SCIENCES; nanofluidics; single particle catalysis; Cu oxidation; CO oxidation; dark field scattering spectroscopy; LSPR; microreactor; nanoreactor; heterogeneous catalysis; plasmonic sensing;

    Sammanfattning : Heterogeneous catalysis is an important cornerstone of modern society with strong ties to the development of sustainable sources of energy and products. Catalysts are typically realized as supported metal nanoparticles that offer active sites that can accelerate chemical reactions by providing energetically more favorable reaction paths. LÄS MER

  4. 4. Kinetics of Nanoparticle Catalysis from First Principles

    Författare :Mikkel Jørgensen; Chalmers tekniska högskola; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; NATURVETENSKAP; NATURAL SCIENCES; NATURVETENSKAP; NATURAL SCIENCES; TEKNIK OCH TEKNOLOGIER; ENGINEERING AND TECHNOLOGY; NATURVETENSKAP; NATURAL SCIENCES; Density functional Theory; Mean field approximation; Acetylene hydrogenation; Kinetic Monte Carlo; CO oxidation; Entropy; Methane oxidation; Heterogeneous catalysis; Kinetic modeling; Nanoparticles;

    Sammanfattning : Modern society depends heavily on heterogeneous catalysis, which creates strong economical and environmental incentives to improve catalyst efficiency. Heterogeneous catalysts are often realized as metal nanoparticles (NPs) supported on oxide surfaces, and catalysts are traditionally developed by trial and error approaches. LÄS MER

  5. 5. Studies of Molecular Interactions with Single Nanoparticles: Combining in Situ Plasmonic Nanospectroscopy with Transmission Electron Microscopy

    Författare :Sara Nilsson; Chalmers tekniska högskola; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; oxidation; plasmonic nanospectroscopy; heterogeneous catalysis; localized surface plasmon resonance sensing; grain boundary; transmission electron microscopy; single nanoparticle; palladium hydride; dark-field scattering spectroscopy;

    Sammanfattning : The cyclic methanol and hydrogen economies are two viable options in the strive for clean energy production. Industrial methanol synthesis is conducted over copper (Cu)-based catalysts. However, Cu is prone to oxidation, which leads to Cu catalyst deactivation. LÄS MER