Sökning: "Molecular photodissociation"

Visar resultat 1 - 5 av 24 avhandlingar innehållade orden Molecular photodissociation.

  1. 1. Atomic and Molecular Dynamics Probed by Intense Extreme Ultraviolet Attosecond Pulses

    Författare :Jasper Peschel; Atomfysik; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; Attosecond science; Ultrafast phenomena; High-order Harmonics Generation; Free Electron Lasers; Photoionization; Photodissociation; Fysicumarkivet A:2021:Peschel;

    Sammanfattning : This thesis work was aimed to investigate dynamical processes in atoms and molecules on ultrafast time scales initiated by absorption of light in the extreme ultraviolet (XUV) regime. In particular, photoionization and photodissociation have been studied using pump-probe techniques involving ultrafast laser pulses. LÄS MER

  2. 2. Investigation of Ultrafast Molecular Dynamics via Covariance Mapping : A Tool for Intense XUV Light Sources

    Författare :Jan Lahl; Atomfysik; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; Covariance; Ultrafast; High-order harmonic generation; Extreme Ultraviolet; Pump probe; FLASH; Velocity map imaging; wavefront; FEL; photodissociation; Coulomb explosion; Fysicumarkivet A:2019:Lahl;

    Sammanfattning : The study of molecular dynamics involves observations of the motion of nuclei and electrons. While nuclear motion is usually on the picosecond or femtosecond timescale, attosecond precision is necessary to directly observe the motion of electrons. LÄS MER

  3. 3. X-ray Absorption and Fragmentationas Initial Steps of Radiation Damage in Free Organic Molecules and Nanoparticles

    Författare :Abdul Rahman Abid; Minna Patanen; Olle Björneholm; Juha Nikkinen; Laurent Nahon; Uppsala universitet; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; Coincidence spectroscopy; PEPI PI CO; electron spectroscopy; X-ray absorption spectroscopy; mass spectrometry; photodissociation; gas-phase; liquids; nanoparticles; charge transfer; synchrotron radiation; Fysik; Physics; Physics with spec. in Atomic; Molecular and Condensed Matter Physics; Fysik med inriktning mot atom- molekyl- och kondenserande materiens fysik;

    Sammanfattning : Understanding the molecular radiation damage is crucial in radiobiology, molecular physics, and atmospheric science. In this thesis, the initial steps of radiation damage of anhydrous gas-phase molecules and hydrated nanoparticles were studied using synchrotron radiation based electron-ion coincidence spectroscopy and X-ray absorption spectroscopy under vacuum conditions. LÄS MER

  4. 4. Ultrafast Photo-induced Reaction Dynamics of Small Molecules

    Författare :Malin Kadi; Jan Davidsson; Eva Åkesson; Sören Keiding; Uppsala universitet; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; Physical chemistry; pump-probe spectroscopy; reaction dynamics; photodissociation; aryl halides; spin-orbit coupling; ab initio calculations; molecular dynamics; vibrational wavepackets; Fysikalisk kemi; Physical chemistry; Fysikalisk kemi;

    Sammanfattning : The main focus of this thesis is the investigation of the dissociation dynamics of aryl halides using femtosecond pump-probe spectroscopy. In the monohalogenated aryl halides, iodo-, bromo- and chlorobenzene, the rate of dissociation following excitation at 266 nm in the gas phase increased with increasing mass of the halogen atom. LÄS MER

  5. 5. Single-photon multiple ionisation of atoms and molecules investigated by coincidence spectroscopy : Site-specific effects in acetaldehyde and carbon dioxide

    Författare :Sergey Zagorodskikh; Raimund Feifel; Vitali Zhaunerchyk; Melanie Mucke; Maria Novella Piancastelli; Tom Field; Uppsala universitet; []
    Nyckelord :NATURVETENSKAP; NATURAL SCIENCES; acetaldehyde; carbon dioxide; xenon; electron correlation; double ionisation; triple ionisation; core-valence ionisation; site-specific Auger decay; multiple Auger decay; branching ratios; site-specific photodissociation; molecular rearrangement; time-of-flight multi-electron-ion coincidence spectroscopy; synchrotron radiation; Physics with spec. in Atomic; Molecular and Condensed Matter Physics; Fysik med inriktning mot atom- molekyl- och kondenserande materiens fysik;

    Sammanfattning : In this thesis, multiple ionisation processes of free atoms and molecules upon single photon absorption are studied by means of a versatile multi-electron-ion coincidence spectroscopy method based on a magnetic bottle, primarily in combination with synchrotron radiation. The latter offered the possibility to access not only valence but also core levels, revealing processes, which promote the target systems into different charge states. LÄS MER